吉林省西部典型高氟区土壤及蔬菜氟分布特征和污染评价

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关键词：氟形态；氟迁移；苏打盐碱化土壤；富集系数；污染评价中图分类号：X53；X825 文献标志码：A 文章编号：1672-2043（2025）09-2296-09 doi：10.11654/jaes.2024-0892

Abstract：Teiofthisseahistoexploretheelatishipetweenfuorefractioninsoilandcontentinvegetabesinteste JiliProviceefluoiedistrbuioofvegetablsinigfuoieareaswillbgaspdesultanprovideteoecaluportfor efectiveuseofagriculturallandandsafeproductionofvegetables.67vegetablesamplesof12typesandtheirzospheresoilsamples， andeightwildplantsamplesoffourtysasontrolswerecolctedfroQian'anountyatypialhighfuorineareainteteJilin Province.Thefuonecontetsinzospersoilandegeablesereanalyd，andteirahiskasevauatedusingthect coficentateoltiodex.sultssoeatalfluoie（T-），watesolubleuoi（Ws-F）hangebleuE F），iron-manganseboudfuoe（FeMn）gacallundfuoi（Or）andresidualfuoeRs）ioseil 202.79-319.12，1.45-9.89，3.49-21.25，6.95-25.72，1.78-5.16 mg kg-1 ， and 174.67-289.97 mg·kg-1 ，respectively， with an average values of 242.74， 4.42， 7.63，12.77， 3.50mg⋅kg-1 and 214.41mg⋅kg-1 ，respectively.Its average content of Ws-F was 1.77 times that of surface soilin fluorosisareas，which wasrelated tothe higherlevel of pH andHCO3 content insoda saline-alkali soils.The content of biologically availablefluorne（Ef-）washigeadingtofuodemoreasilytranferedfrosoiltoegeables.Thfuorinecontentingeables ranged from 0.21 mg·kg-1 to 8.89mg⋅kg-1 .The order of fluorine content and enrichment coefficients in different parts was leaves>fruits.It wasmoredetailedinteoderoffuityvegetables>leafvegetables>fruits.ereasasignificantlypositiverelatioshipetweefuoin in vegetables and Ws-F in the soil except eggplants.Fluorine content in 40.00% of the tested vegetables exceeded the national standard（1 mg kg-1 ）.Theresultsofhealthriskassessmentindicatedthatbiterletuceposedacertainrisktochildren'shalth.Thecontentof Ws-F andEx-Finsodasaline-alkalisoilwashighanditsbioavailabilitywasstrong，whichcausedthefluorinecontent insomevegetables excedingthenationalhealthstandards.Fruityvegetableswithlowerfluorineenrichmentcoeffcientarerecommendedtobeplantedto decline fluoride health risks.

Keywords：fluorinespeciation;fluorine migration;sodasaline-alkalisoil;enrichmentcoeficient;contaminationevaluation

吉林省西部早在1964年就被确定为北方典型干旱、半干旱饮水型潜水高氟地氟病区，当地患氟斑牙、氟骨病的病人较多。（剩余16291字）