CaO2调控潜育化稻田CH4排放的动态特征及机制

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关键词:潜育化稻田;过氧化钙;产 CH4 菌;CH4氧化菌;CH4排放中图分类号:X71;S511 文献标志码:A 文章编号:1672-2043(2025)11-2994-11 doi:10.11654/jaes.2024-1091
Abstract:Long-termwaterlogingingleizationpaddyfieldscreatesanaerobicsoilconditionsthatpromotesubstantialacuulationof reductivesubstance,whichnotonlyimpedesricegrowthbutalsoexacerbates methane(CH4)eisions.Toadressthisissealcium peroxide( CaO2 ) granules(2-3 mm diameter) prepared through disc granulation were applied to investigate their impacts on CH .4 emissions andunderlying mechanisms undercontiuousflooding.Apotexperimentwithfourtreatments asconducted:control(CK),andthree CaO2 application rates (LC: 0.15 g⋅kg-1 ,MC: 0.30 g⋅kg-1 ,HC: 0.60 g⋅kg-1 ,freshsoil basis). Systematic analyses were performed on soil physicochemicalproptisductiesubstancsrobialfunctioalgenbundc,ndCHisios.Kefdingsevealedl (204号 CaO2 treatments initially suppressed CH .4 emissions within 43 days after transplanting,but ultimately enhanced emissions by maturity. The MC treatment showed 88.2% higher cumulative emissions than CK, though 29.2% and 10.4% lower than LC and HC treatments respectively.LC treatment demonstrated superior reduction efficiency for total reductive substances ( 0.1% ),active reductive substances ( 0.6% ),F e2+(3.0%) ,and Mn2+(8.2% )compared to CK.Methanogen(mcrA) gene abundance increased across alltreatments ( LC>HC> MC),while methanotroph(pmoA) abundance decreased in LC,MC but increased in HC. CaO2 amendments elevated soil pH and dissolved organic carbon(DOC), while reducing NH4-N and NOj-N contents.These findings indicate that CaO2 application can temporarily mitigate (204号 CH4 emissions within 43 days,but exhibits complex long-term dynamics.
Keywords:submerged rice soil; calcium peroxide;methanogens;methanotrophs; CH4 emission
甲烷( CH4 )是仅次于二氧化碳( CO2 )的第二大温室气体,其百年全球增温潜势(GWP)是 CO2 的27.9倍,具有很强的温室效应1。(剩余22110字)